Toye is a surname. Notable people with the surname include:

• Alfred Toye (1897–1955), British World War I veteran
• Christy Toye (born 1983), Irish sportsperson
• Clive Toye (born 1932), British-American sports journalist
• Francis Toye (1883–1964), English music critic, teacher, writer and educational administrator
• Frederick E.O. Toye (born 1967), American television director and producer
• Geoffrey Toye (1889–1942), British conductor, composer and opera producer
• Joe Toye (1919-1995), American World War II veteran prominently featured in the book and TV miniseries Band of Brothers
• John Toye (c. 1936–1992), British presenter and newsreader
• John Toye (economist) (1942-2021), British economist
• Lori Toye, American New Age author
• Mason Toye (born 1998), American soccer player
• Patrice Toye (born 1967), Belgian film director
• Richard Toye (born 1973), British historian
• Robert Toye, American bank robber
• Wendy Toye (1917–2010), British dancer, stage and film director and actress
• William J. Toye (1931–2018), American art forger